Chemo-mechanical modification of cottonwood for Pb(2+) removal from aqueous solutions: Sorption mechanisms and potential application as biofilter in drip-irrigation.
Identifieur interne : 001970 ( Main/Exploration ); précédent : 001969; suivant : 001971Chemo-mechanical modification of cottonwood for Pb(2+) removal from aqueous solutions: Sorption mechanisms and potential application as biofilter in drip-irrigation.
Auteurs : Ahmed Mosa [Égypte] ; Ayman El-Ghamry [Égypte] ; Peter Trüby [Allemagne] ; Mahmoud Omar [Égypte] ; Bin Gao [États-Unis] ; Abdelhamid Elnaggar [Égypte] ; Yuncong Li [États-Unis]Source :
- Chemosphere [ 1879-1298 ] ; 2016.
Descripteurs français
- KwdFr :
- Adsorption (MeSH), Biomasse (MeSH), Cinétique (MeSH), Composés du potassium (composition chimique), Eaux usées (composition chimique), Hydroxydes (composition chimique), Irrigation agricole (MeSH), Microscopie électronique à balayage (MeSH), Plomb (analyse), Polluants chimiques de l'eau (analyse), Populus (composition chimique), Propriétés de surface (MeSH), Raphanus (croissance et développement), Sol (composition chimique), Solutions (MeSH), Spectrométrie d'émission X (MeSH), Spectroscopie infrarouge à transformée de Fourier (MeSH).
- MESH :
- analyse : Plomb, Polluants chimiques de l'eau.
- composition chimique : Composés du potassium, Eaux usées, Hydroxydes, Populus, Sol.
- croissance et développement : Raphanus.
- Adsorption, Biomasse, Cinétique, Irrigation agricole, Microscopie électronique à balayage, Propriétés de surface, Solutions, Spectrométrie d'émission X, Spectroscopie infrarouge à transformée de Fourier.
English descriptors
- KwdEn :
- Adsorption (MeSH), Agricultural Irrigation (MeSH), Biomass (MeSH), Hydroxides (chemistry), Kinetics (MeSH), Lead (analysis), Microscopy, Electron, Scanning (MeSH), Populus (chemistry), Potassium Compounds (chemistry), Raphanus (growth & development), Soil (chemistry), Solutions (MeSH), Spectrometry, X-Ray Emission (MeSH), Spectroscopy, Fourier Transform Infrared (MeSH), Surface Properties (MeSH), Waste Water (chemistry), Water Pollutants, Chemical (analysis).
- MESH :
- chemical , analysis : Lead, Water Pollutants, Chemical.
- chemical , chemistry : Hydroxides, Potassium Compounds, Soil, Waste Water.
- chemistry : Populus.
- growth & development : Raphanus.
- Adsorption, Agricultural Irrigation, Biomass, Kinetics, Microscopy, Electron, Scanning, Solutions, Spectrometry, X-Ray Emission, Spectroscopy, Fourier Transform Infrared, Surface Properties.
Abstract
Using biomass (e.g. crop residues) and its derivatives as biosorbents have been recognized as an eco-friendly technique for wastewater decontamination. In this study, mechanically modified cottonwood was further activated with KOH to improve its sorption of Pb(2+). In addition, its potential as a biofilter to safeguard radish (Raphanus sativus, L.) against Pb-stress was evaluated in a gravity-fed drip irrigation system. Physiochemical properties of the chemo-mechanically activated cottonwood (CMACW) and the mechanically activated cottonwood (MACW) before and after sorption process were characterized using scanning electron microscopy (SEM), energy dispersive X-ray spectroscopy (EDS), transmission electron microscopy (TEM), digital selected-area electron diffraction (SAED) and Fourier transform infrared spectroscopy (FTIR). After activation, several sorption mechanisms (i.e. precipitation, electrostatic outer- and inner-sphere complexation) were responsible for the higher sorption capacity of CMACW as compared with MACW (8.55 vs. 7.28 mg g(-1)). Sorption kinetics and isotherms fitted better with the pseudo-second-order and Langmuir models as compared with the pseudo-first-order and Freundlich models, respectively. In the gravity-fed drip irrigation system, the CMACW biofilter reduced the accumulation of Pb in radish roots and shoots and avoided reaching the toxic limits in some cases. Soil types had a significant effect on Pb(2+) bioavailability because of the difference in sorption ability. Findings from this study showed that CMACW biofilter can be used as a safeguard for wastewater irrigation.
DOI: 10.1016/j.chemosphere.2016.06.101
PubMed: 27393935
Affiliations:
- Allemagne, Égypte, États-Unis
- Bade-Wurtemberg, District de Fribourg-en-Brisgau, Floride
- Fribourg-en-Brisgau
Links toward previous steps (curation, corpus...)
Le document en format XML
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Soil and Water Science Department, University of Florida, Gainesville, FL 32611, United States.</nlm:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>Tropical Research and Education Center, University of Florida, Homestead, FL 33031, United States; Soil and Water Science Department, University of Florida, Gainesville, FL 32611</wicri:regionArea><placeName><region type="state">Floride</region></placeName></affiliation></author></analytic><series><title level="j">Chemosphere</title><idno type="eISSN">1879-1298</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Adsorption (MeSH)</term><term>Agricultural Irrigation (MeSH)</term><term>Biomass (MeSH)</term><term>Hydroxides (chemistry)</term><term>Kinetics (MeSH)</term><term>Lead (analysis)</term><term>Microscopy, Electron, Scanning (MeSH)</term><term>Populus (chemistry)</term><term>Potassium Compounds (chemistry)</term><term>Raphanus (growth & development)</term><term>Soil (chemistry)</term><term>Solutions (MeSH)</term><term>Spectrometry, X-Ray Emission (MeSH)</term><term>Spectroscopy, Fourier Transform Infrared (MeSH)</term><term>Surface Properties (MeSH)</term><term>Waste Water (chemistry)</term><term>Water Pollutants, Chemical (analysis)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Adsorption (MeSH)</term><term>Biomasse (MeSH)</term><term>Cinétique (MeSH)</term><term>Composés du potassium (composition chimique)</term><term>Eaux usées (composition chimique)</term><term>Hydroxydes (composition chimique)</term><term>Irrigation agricole (MeSH)</term><term>Microscopie électronique à balayage (MeSH)</term><term>Plomb (analyse)</term><term>Polluants chimiques de l'eau (analyse)</term><term>Populus (composition chimique)</term><term>Propriétés de surface (MeSH)</term><term>Raphanus (croissance et développement)</term><term>Sol (composition chimique)</term><term>Solutions (MeSH)</term><term>Spectrométrie d'émission X (MeSH)</term><term>Spectroscopie infrarouge à transformée de Fourier (MeSH)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="analysis" xml:lang="en"><term>Lead</term><term>Water Pollutants, Chemical</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Hydroxides</term><term>Potassium Compounds</term><term>Soil</term><term>Waste Water</term></keywords><keywords scheme="MESH" qualifier="analyse" xml:lang="fr"><term>Plomb</term><term>Polluants chimiques de l'eau</term></keywords><keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Populus</term></keywords><keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Composés du potassium</term><term>Eaux usées</term><term>Hydroxydes</term><term>Populus</term><term>Sol</term></keywords><keywords scheme="MESH" qualifier="croissance et développement" xml:lang="fr"><term>Raphanus</term></keywords><keywords scheme="MESH" qualifier="growth & development" xml:lang="en"><term>Raphanus</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Adsorption</term><term>Agricultural Irrigation</term><term>Biomass</term><term>Kinetics</term><term>Microscopy, Electron, Scanning</term><term>Solutions</term><term>Spectrometry, X-Ray Emission</term><term>Spectroscopy, Fourier Transform Infrared</term><term>Surface Properties</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Adsorption</term><term>Biomasse</term><term>Cinétique</term><term>Irrigation agricole</term><term>Microscopie électronique à balayage</term><term>Propriétés de surface</term><term>Solutions</term><term>Spectrométrie d'émission X</term><term>Spectroscopie infrarouge à transformée de Fourier</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Using biomass (e.g. crop residues) and its derivatives as biosorbents have been recognized as an eco-friendly technique for wastewater decontamination. In this study, mechanically modified cottonwood was further activated with KOH to improve its sorption of Pb(2+). In addition, its potential as a biofilter to safeguard radish (Raphanus sativus, L.) against Pb-stress was evaluated in a gravity-fed drip irrigation system. Physiochemical properties of the chemo-mechanically activated cottonwood (CMACW) and the mechanically activated cottonwood (MACW) before and after sorption process were characterized using scanning electron microscopy (SEM), energy dispersive X-ray spectroscopy (EDS), transmission electron microscopy (TEM), digital selected-area electron diffraction (SAED) and Fourier transform infrared spectroscopy (FTIR). After activation, several sorption mechanisms (i.e. precipitation, electrostatic outer- and inner-sphere complexation) were responsible for the higher sorption capacity of CMACW as compared with MACW (8.55 vs. 7.28 mg g(-1)). Sorption kinetics and isotherms fitted better with the pseudo-second-order and Langmuir models as compared with the pseudo-first-order and Freundlich models, respectively. In the gravity-fed drip irrigation system, the CMACW biofilter reduced the accumulation of Pb in radish roots and shoots and avoided reaching the toxic limits in some cases. Soil types had a significant effect on Pb(2+) bioavailability because of the difference in sorption ability. Findings from this study showed that CMACW biofilter can be used as a safeguard for wastewater irrigation. </div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Curated" Owner="NLM"><PMID Version="1">27393935</PMID><DateCompleted><Year>2017</Year><Month>02</Month><Day>15</Day></DateCompleted><DateRevised><Year>2018</Year><Month>12</Month><Day>02</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1879-1298</ISSN><JournalIssue CitedMedium="Internet"><Volume>161</Volume><PubDate><Year>2016</Year><Month>Oct</Month></PubDate></JournalIssue><Title>Chemosphere</Title><ISOAbbreviation>Chemosphere</ISOAbbreviation></Journal><ArticleTitle>Chemo-mechanical modification of cottonwood for Pb(2+) removal from aqueous solutions: Sorption mechanisms and potential application as biofilter in drip-irrigation.</ArticleTitle><Pagination><MedlinePgn>1-9</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0045-6535(16)30869-4</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.chemosphere.2016.06.101</ELocationID><Abstract><AbstractText>Using biomass (e.g. crop residues) and its derivatives as biosorbents have been recognized as an eco-friendly technique for wastewater decontamination. In this study, mechanically modified cottonwood was further activated with KOH to improve its sorption of Pb(2+). In addition, its potential as a biofilter to safeguard radish (Raphanus sativus, L.) against Pb-stress was evaluated in a gravity-fed drip irrigation system. Physiochemical properties of the chemo-mechanically activated cottonwood (CMACW) and the mechanically activated cottonwood (MACW) before and after sorption process were characterized using scanning electron microscopy (SEM), energy dispersive X-ray spectroscopy (EDS), transmission electron microscopy (TEM), digital selected-area electron diffraction (SAED) and Fourier transform infrared spectroscopy (FTIR). After activation, several sorption mechanisms (i.e. precipitation, electrostatic outer- and inner-sphere complexation) were responsible for the higher sorption capacity of CMACW as compared with MACW (8.55 vs. 7.28 mg g(-1)). Sorption kinetics and isotherms fitted better with the pseudo-second-order and Langmuir models as compared with the pseudo-first-order and Freundlich models, respectively. In the gravity-fed drip irrigation system, the CMACW biofilter reduced the accumulation of Pb in radish roots and shoots and avoided reaching the toxic limits in some cases. Soil types had a significant effect on Pb(2+) bioavailability because of the difference in sorption ability. Findings from this study showed that CMACW biofilter can be used as a safeguard for wastewater irrigation. </AbstractText><CopyrightInformation>Copyright © 2016 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Mosa</LastName><ForeName>Ahmed</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>Soils Department, Faculty of Agriculture, Mansoura University, 35516 Mansoura, Egypt.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>El-Ghamry</LastName><ForeName>Ayman</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>Soils Department, Faculty of Agriculture, Mansoura University, 35516 Mansoura, Egypt.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Trüby</LastName><ForeName>Peter</ForeName><Initials>P</Initials><AffiliationInfo><Affiliation>Institute of Soil Science and Forest Nutrition, Freiburg University, Freiburg, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Omar</LastName><ForeName>Mahmoud</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>Soils Department, Faculty of Agriculture, Mansoura University, 35516 Mansoura, Egypt.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Gao</LastName><ForeName>Bin</ForeName><Initials>B</Initials><AffiliationInfo><Affiliation>Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL 32611, United States. Electronic address: bg55@ufl.edu.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Elnaggar</LastName><ForeName>Abdelhamid</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>Soils Department, Faculty of Agriculture, Mansoura University, 35516 Mansoura, Egypt.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Li</LastName><ForeName>Yuncong</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Tropical Research and Education Center, University of Florida, Homestead, FL 33031, United States; Soil and Water Science Department, University of Florida, Gainesville, FL 32611, United States.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2016</Year><Month>07</Month><Day>07</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Chemosphere</MedlineTA><NlmUniqueID>0320657</NlmUniqueID><ISSNLinking>0045-6535</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D006878">Hydroxides</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D017680">Potassium Compounds</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D012987">Soil</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D012996">Solutions</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D062065">Waste Water</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D014874">Water Pollutants, Chemical</NameOfSubstance></Chemical><Chemical><RegistryNumber>2P299V784P</RegistryNumber><NameOfSubstance UI="D007854">Lead</NameOfSubstance></Chemical><Chemical><RegistryNumber>WZH3C48M4T</RegistryNumber><NameOfSubstance UI="C029943">potassium hydroxide</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000327" MajorTopicYN="N">Adsorption</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D057914" MajorTopicYN="Y">Agricultural Irrigation</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D018533" MajorTopicYN="N">Biomass</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D006878" MajorTopicYN="N">Hydroxides</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D007700" MajorTopicYN="N">Kinetics</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D007854" MajorTopicYN="N">Lead</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="Y">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D008855" MajorTopicYN="N">Microscopy, Electron, Scanning</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D032107" MajorTopicYN="N">Populus</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D017680" MajorTopicYN="N">Potassium Compounds</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D031224" MajorTopicYN="N">Raphanus</DescriptorName><QualifierName UI="Q000254" MajorTopicYN="Y">growth & development</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D012987" MajorTopicYN="N">Soil</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D012996" MajorTopicYN="N">Solutions</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D013052" MajorTopicYN="N">Spectrometry, X-Ray Emission</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D017550" MajorTopicYN="N">Spectroscopy, Fourier Transform Infrared</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D013499" MajorTopicYN="N">Surface Properties</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D062065" MajorTopicYN="N">Waste Water</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D014874" MajorTopicYN="N">Water Pollutants, Chemical</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="Y">analysis</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Biofilter</Keyword><Keyword MajorTopicYN="N">Chemical modification</Keyword><Keyword MajorTopicYN="N">Cottonwood</Keyword><Keyword MajorTopicYN="N">Mechanical modification</Keyword><Keyword MajorTopicYN="N">Radish</Keyword><Keyword MajorTopicYN="N">Soil</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2016</Year><Month>04</Month><Day>07</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2016</Year><Month>06</Month><Day>10</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2016</Year><Month>06</Month><Day>27</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2016</Year><Month>7</Month><Day>10</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2016</Year><Month>7</Month><Day>10</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2017</Year><Month>2</Month><Day>16</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">27393935</ArticleId><ArticleId IdType="pii">S0045-6535(16)30869-4</ArticleId><ArticleId IdType="doi">10.1016/j.chemosphere.2016.06.101</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Allemagne</li><li>Égypte</li><li>États-Unis</li></country><region><li>Bade-Wurtemberg</li><li>District de Fribourg-en-Brisgau</li><li>Floride</li></region><settlement><li>Fribourg-en-Brisgau</li></settlement></list><tree><country name="Égypte"><noRegion><name sortKey="Mosa, Ahmed" sort="Mosa, Ahmed" uniqKey="Mosa A" first="Ahmed" last="Mosa">Ahmed Mosa</name></noRegion><name sortKey="El Ghamry, Ayman" sort="El Ghamry, Ayman" uniqKey="El Ghamry A" first="Ayman" last="El-Ghamry">Ayman El-Ghamry</name><name sortKey="Elnaggar, Abdelhamid" sort="Elnaggar, Abdelhamid" uniqKey="Elnaggar A" first="Abdelhamid" last="Elnaggar">Abdelhamid Elnaggar</name><name sortKey="Omar, Mahmoud" sort="Omar, Mahmoud" uniqKey="Omar M" first="Mahmoud" last="Omar">Mahmoud Omar</name></country><country name="Allemagne"><region name="Bade-Wurtemberg"><name sortKey="Truby, Peter" sort="Truby, Peter" uniqKey="Truby P" first="Peter" last="Trüby">Peter Trüby</name></region></country><country name="États-Unis"><region name="Floride"><name sortKey="Gao, Bin" sort="Gao, Bin" uniqKey="Gao B" first="Bin" last="Gao">Bin Gao</name></region><name sortKey="Li, Yuncong" sort="Li, Yuncong" uniqKey="Li Y" first="Yuncong" last="Li">Yuncong Li</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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